Yes, you simply select the ports you wish to aggregate and apply.
The Cisco Catalyst side requires matching VLAN config and LACP Active or Passive mode.
Removing ports from aggregation involves selecting the ports and clicking "split" in the Meraki dashboard, and removing the port-channel config from the Cisco switch side.
Note: I would shut down all links in the bundle except for 1 to avoid introducing any potentials of loops.
More information can be found in the following doc - Link Aggregation and Load Balancing - Cisco Meraki